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Suppression of ferromagnetism and emergence of spin-glass-like behavior in the CuCr2-xSnx S2Se2 spinels
dc.contributor.author | Pardo-Sainz, Miguel | |
dc.contributor.author | Moris, Silvana | |
dc.contributor.author | Piquer, Cristina | |
dc.contributor.author | Rodríguez-Velamazán, José Alberto | |
dc.contributor.author | López, María Luisa | |
dc.contributor.author | Álvarez-Serrano, Inmaculada | |
dc.contributor.author | Galdámez, Antonio | |
dc.contributor.author | Campo, Javier | |
dc.date.accessioned | 2024-10-17T15:36:48Z | |
dc.date.available | 2024-10-17T15:36:48Z | |
dc.date.issued | 2024 | |
dc.identifier.uri | http://repositorio.ucm.cl/handle/ucm/5737 | |
dc.description.abstract | Magnetometry, neutron diffraction experiments, and high-resolution transmission electron microscopy (HRTEM) were performed to study the magnetic behavior of CuCr2−𝑥Sn𝑥S2Se2 (0.2≤𝑥≤1.0) solid solutions and experimentally determine the appropriate magnetic structure for these systems. For all samples, the main phase with normal spinel-type structure (𝐹𝑑‾3 𝑚) was refined. For low Sn concentration a minority monoclinic phase appears also corroborated with HRTEM analyses. Together with the results from magnetization experiments, neutron diffraction measurements allowed to establish that for samples with 𝑥≤0.4 there is a ferromagnetic long-range order at high temperatures labeled with the 3𝑑 irrep mΓ+4 of 𝐹𝑑‾3𝑚.1′, while for 𝑥>0.4 no magnetic signal is observed, indicating that the ferromagnetic behavior is suppressed and replaced with a spin-glass-like state. | es_CL |
dc.language.iso | en | es_CL |
dc.rights | Atribución-NoComercial-SinDerivadas 3.0 Chile | * |
dc.rights.uri | http://creativecommons.org/licenses/by-nc-nd/3.0/cl/ | * |
dc.source | Physical Review B, 110(6), 064436 | es_CL |
dc.title | Suppression of ferromagnetism and emergence of spin-glass-like behavior in the CuCr2-xSnx S2Se2 spinels | es_CL |
dc.type | Article | es_CL |
dc.ucm.indexacion | Scopus | es_CL |
dc.ucm.indexacion | Isi | es_CL |
dc.ucm.uri | journals.aps.org/prb/abstract/10.1103/PhysRevB.110.064436 | es_CL |
dc.ucm.doi | doi.org/10.1103/PhysRevB.110.064436 | es_CL |
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